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38 Relationship between island density and coverage during the four steps of p-6P ultrathin film growth. 088/mm2, respectively [21]. L. , “Ultrathin-film growth of para-sexiphenyl (I): submonolayer thin-film growth as a function of the substrate temperature,” Journal of Physical Chemistry B, 112(26), 7816, 2008. ) (b) Third and fourth steps: the small gray-shadowed area in (b) is expanded and shown in detail in (a) [22]. L. , “Ultrathin-film growth of parasexiphenyl (II): formation of large-size domain and continuous thin film,” Journal of Physical Chemistry B, 112(26), 7821, 2008.
5 nm H2Pc thin films grown on p-6P ultrathin film (3 nm). ZnPc and H2Pc crystals take on several in-plane orientations on the p-6P monolayer film and only one in-plane orientation on the p-6P double layer film [29]. L. , “Weak epitaxy growth of metal-free phthalocyanine on p-sexiphenyl monolayer and double-layer films,” Journal of Physical Chemistry B, 112(10), 3132, 2008. 5 nm H2Pc grown on p-6P (a) monolayer film and (b) double layer film, respectively. H2Pc crystals exhibit three in-plane orientations on the p-6P monolayer film and only one in-plane orientation on the p-6P double layer film [29].
The thermodynamically metastable monolayer is transiting to thermodynamically stable double layer. The transition rate is about equal to the growth rate of monolayer [22]. L. , “Ultrathin-film growth of para-sexiphenyl (II): formation of large-size domain and continuous thin film,” Journal of Physical Chemistry B, 112(26), 7821, 2008. ) critical nucleus and a stable nucleus when meeting. The low island density supplies the precondition for the formation of large-size domains. During the growth process of monolayer islands, new molecules or molecular clusters should nucleate on each domain.