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The effect of structural rigidity was also demonstrated quantitatively on a series of As–S glasses exposed to different dosages of 60Co radiation [40]. 19a shows the enthalpy release ΔH of glasses exposed to cumulative doses of 3 MGy and 4 MGy compared to that of unexposed glasses. All samples had been stored in the dark at room temperature for 38 months prior to irradiation. 19 (a) Comparison of the enthalpy release ΔH of As–S glasses irradiated with 3 MGy and 4 MGy and maintained in the dark. (b) Glass transition temperature Tg measured at 10°C/min of As–S glasses as a function of the mean coordination
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The trends for both systems show a clear minimum in fragility at the rigidity percolation threshold. 7 Dependence of the fragility index, m, on the average coordination